Kerry Park is your must-do photo op. it sits high on a hill northwest of downtown and affords an excellent view of downtown, Elliot Bay, and Mt. Rainier if conditions are favorable.
The Ride the Ducks tour of Seattle is really good. It’s a tour riding on a WWII-era amphibious vehicle and runs on land and water. Fun stuff.
You can also book orca whale watching tours through a few companies, but the Seattle aquarium has a nice one, too. There are three resident pods of whales that live in Puget Sound (mostly north around the San Juan Islands), and the companies all work together to locate them, so it’s pretty reliable. Plus, you’ll get to see bald eagles and other wildlife.