It looks like DUI, Theft (“Larceny”), and Assault are the top 3…
Disorderly conduct and Marijuana possession seem be come out pretty close along with Drunkenness and Liquor Laws (I’m assuming this is underage drinking, permitting laws, things along those lines?)
This is all for 2005, didn’t find newer stats during a quick search
Publicly available data for NYC shows assault tops arrest lists.
Marijuana-related arrests were among the top five until a few years ago when those crimes were de-prioritized and even more as it has become de-criminalized.